It's tough off the top of the head, but the more I think about it, Mysterio accomplished a lot in both WCW and WWE for a long time. Rob Van Dam accomplished a lot in ECW, but treaded water for a while in WWE.
Mysterio didn't tread water far as much in WWE unless you count all the injuries. Up until about the time Sin Cara came around and Mysterio teamed with him Mysterio was involved in (unless he was injured) an upper card program and it was normally one of the more entertaining ones. And he always did very well in them.
Rob Van Dam's programs weren't always as interesting even though they did result in some entertaining matches.
Plus I think Mysterio's legendary work in WCW is better than Rob's legendary work in ECW.
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