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That one was called Hush. Probably the best ep they ever did. The one with Angel killing Jenny is called Passion, also an awesome episode.
Others:
-Fool For Love (season 5, when Spike recounts his history)
-Pretty much all of Season 3 (Eliza Dushku is teh sex)
-Storyteller (S7, where Andrew narrates a day via camcorder)
-End of S5 was pretty good (dies saving the world...should've been the real ending IMO)
Having said that, the show was pretty much made up of smaller moment after smaller moment, so a list would be humongous.
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